Well as Betty Boop said, Kefka because he actually did take over the world. but it was a shame he was made to be comic relief so often. I also liked Edea/Ultimecia, both of them were pretty cool, especially since they're the only major female villains that come to mind (Although if I'm mistaken, doesn't FFII have a female antagonist?). Jenova (oh there we go, this is another female villain) is also up there, mostly because she was utterly silent, yet was the the mastermind behind the whole plot of FFVII
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